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A polariton filter turns ordinary laser light into quantum light

Nature Materials paper Tuesday, 19 February 2019

Artist’s impression of the polaritonic photon conversion platform. Laser photons enter through the top mirror and leave through the bottom mirror exhibiting quantum ‘granularity’ – after interacting with the semiconductor layer. Image: Andrew Wood

An international team of researchers led out of Macquarie University has demonstrated a new approach for converting ordinary laser light into genuine quantum light.

Their approach uses nanometre-thick films made of gallium arsenide, which is a semiconductor material widely used in solar cells. They sandwich the thin films between two mirrors to manipulate the incoming photons.

The photons interact with electron-hole pairs in the semiconductor, forming new chimeric particles called polaritons that carry properties from both the photons and the electron-hole pairs. The polaritons decay after a few picoseconds, and the photons they release exhibit distinct quantum signatures.

The teams’ research was published overnight in the journal Nature Materials.

While these quantum signatures are weak at the moment, the work opens up a new avenue for producing single photons on demand.

“The ability to produce single photons on demand is hugely important for future applications in quantum communication and optical quantum information processing,” says Associate Professor Thomas Volz from the Department of Physics and Astronomy and the senior author on the paper. “Think unbreakable encryption, super-fast computers, more efficient computer chips or even optical transistors with minimal power consumption.”

Currently single-photon emitters are typically created by materials engineering—where the material itself is assembled in such a way that the ‘quantum’ behaviour is built in.

But this standard approach faces serious limitations at smaller and smaller scales because producing identical single-photon emitters by pure materials engineering is extremely challenging.

“This means our approach could be much more amenable for massively scaling up, once we’re able to increase the strength of the quantum signatures we’re producing. We might be able to make identical quantum emitters from semiconductors by photon nanostructure engineering, rather than by direct materials engineering,” says Dr Guillermo Munoz Matutano, also from Macquarie and lead author of the paper.

“While real-world applications are still a fair bit away, our paper describes a major milestone that the polariton community in particular has been waiting on for the last ten to fifteen years. The regime in which polaritons interact so strongly that they can imprint quantum signatures on photons has not been accessed to date and opens up a whole new playground for researchers in the field,” says Thomas.

The Macquarie University team is part of the ARC Centre of Excellence for Engineered Quantum Systems (EQUS), and the experiments were carried out at the CSIRO labs in Lindfield where part of the Macquarie quantum labs are based at present. The paper appears alongside a similar study carried out in parallel at ETH Zurich.

Muñoz-Matutano G, Wood A, Johnsson M, Vidal X, Baragiola BQ, Reinhard A, Lemaître A, Bloch J, Amo A, Nogues G, Besga B, Richard M & Volz T. Emergence of quantum correlations from interacting fibre-cavity polaritons. Nature Materials. February 2019.

Abstract

Emergence of quantum correlations from interacting fibre-cavity polaritons

Over the past decade, exciton-polaritons in semiconductor microcavities have revealed themselves as one of the richest realizations of a light-based quantum fluid, subject to fascinating new physics and potential applications. For instance, in the regime of large two-body interactions, polaritons can be used to manipulate the quantum properties of a light field. In this work, we report on the emergence of quantum correlations in laser light transmitted through a fibre-cavity polariton system. We observe a dispersive shape of the autocorrelation function around the polariton resonance that indicates the onset of this regime. The weak amplitude of these correlations indicates a state that still remains far from a low-photon number state. Nonetheless, given the underlying physical mechanism, our work opens up the prospect of eventually using polaritons to turn laser light into single photons.

Authors

Guillermo Muñoz-Matutano1,2, Andrew Wood1,2, Mattias Johnsson1,2, Xavier Vidal 1,2, Ben Q. Baragiola1,2,3, Andreas Reinhard1,2, Aristide Lemaître4, Jacqueline Bloch4, Alberto Amo5, Gilles Nogues6, Benjamin Besga1,2,6, Maxime Richard1,6 and Thomas Volz1,2

Affiliations

  1. Department of Physics and Astronomy, Macquarie University, Sydney, New South Wales, Australia.
  2. ARC Centre of Excellence for Engineered Quantum Systems, Macquarie University, Sydney, New South Wales, Australia.
  3. ARC Centre for Quantum Computation and Communication Technology, School of Science, RMIT University, Melbourne, Victoria, Australia.
  4. Centre de Nanosciences et de Nanotechnologies, CNRS (C2N), Universities Paris-Sud and Paris-Saclay, Palaiseau, France.
  5. Univ. Lille, CNRS, UMR 8523, PhLAM – Physique des Lasers Atomes et Molécules, Lille, France.
  6. Univ. Grenoble Alpes, CNRS, Grenoble INP, Institut Néel, Grenoble, France